TY - JOUR
T1 - Use of electron microscopy to determine presence of coal dust in a neighborhood bordering an open-air coal terminal in Curtis Bay, Baltimore, Maryland, USA
AU - Aubourg, Matthew A.
AU - Livi, Kenneth J.T.
AU - Sawtell, Gregory G.
AU - Sanchez-Gonzalez, Carlos C.
AU - Spada, Nicholas J.
AU - Dickerson, Russell R.
AU - Chiou, Wen An
AU - Kamanzi, Conchita
AU - Ramachandran, Gurumurthy
AU - Rule, Ana M.
AU - Heaney, Christopher D.
N1 - Publisher Copyright:
© 2024 The Authors
PY - 2024/12/20
Y1 - 2024/12/20
N2 - Background: Despite decreasing US consumption, over 90 million metric tons of coal were exported by the US in 2023, requiring significant infrastructure for transport, handling, and storage of coal at export terminals. Residents in Curtis Bay, Baltimore, Maryland, USA live at the fenceline of an open-air coal terminal and have, for decades, reported rapid accumulation of black dust at their homes. Community-level exposure to coal dust originating from coal handling and storage terminals has remained largely unexplored. Objectives: To investigate community-identified concerns and use a community-driven approach to determine the presence/absence of coal dust on Curtis Bay surfaces. Methods: Passive settled dust samples were collected from two residential areas, 345 m and 1235 m from the coal terminal, using conductive carbon tape. Scanning electron microscopy and energy dispersive X-ray spectroscopy (SEM-EDX) of standard reference coal material and positive control material from the coal terminal in Curtis Bay were used to optimize the morphological and elemental classification criteria for coal dust. A manual SEM-EDX protocol was developed to identify coal particles in settled dust collected on conductive carbon tape in community settings. Results: SEM-EDX analysis confirmed presence of coal dust sampled at both residential locations. Estimated coal dust particle loading at the proximal and distal site were 13.2 and 3.4 coal particles/mm2, respectively. The coal dust particles identified met specific criteria, including size (>5 μm), morphology, and elemental composition (≥75 % carbon, ≤20 % oxygen). Discussion: These findings are consistent with longstanding community concerns and lived experiences regarding the presence of coal dust in Curtis Bay, which neighbors a major open-air coal terminal. This approach has potential for other communities neighboring coal terminals to assess similar concerns with residential coal dust exposure.
AB - Background: Despite decreasing US consumption, over 90 million metric tons of coal were exported by the US in 2023, requiring significant infrastructure for transport, handling, and storage of coal at export terminals. Residents in Curtis Bay, Baltimore, Maryland, USA live at the fenceline of an open-air coal terminal and have, for decades, reported rapid accumulation of black dust at their homes. Community-level exposure to coal dust originating from coal handling and storage terminals has remained largely unexplored. Objectives: To investigate community-identified concerns and use a community-driven approach to determine the presence/absence of coal dust on Curtis Bay surfaces. Methods: Passive settled dust samples were collected from two residential areas, 345 m and 1235 m from the coal terminal, using conductive carbon tape. Scanning electron microscopy and energy dispersive X-ray spectroscopy (SEM-EDX) of standard reference coal material and positive control material from the coal terminal in Curtis Bay were used to optimize the morphological and elemental classification criteria for coal dust. A manual SEM-EDX protocol was developed to identify coal particles in settled dust collected on conductive carbon tape in community settings. Results: SEM-EDX analysis confirmed presence of coal dust sampled at both residential locations. Estimated coal dust particle loading at the proximal and distal site were 13.2 and 3.4 coal particles/mm2, respectively. The coal dust particles identified met specific criteria, including size (>5 μm), morphology, and elemental composition (≥75 % carbon, ≤20 % oxygen). Discussion: These findings are consistent with longstanding community concerns and lived experiences regarding the presence of coal dust in Curtis Bay, which neighbors a major open-air coal terminal. This approach has potential for other communities neighboring coal terminals to assess similar concerns with residential coal dust exposure.
KW - Coal dust
KW - Coal terminal
KW - Community-driven research
KW - Dust characterization
KW - Environmental justice
KW - SEM-EDX
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U2 - 10.1016/j.scitotenv.2024.176842
DO - 10.1016/j.scitotenv.2024.176842
M3 - Article
C2 - 39396779
AN - SCOPUS:85209545860
SN - 0048-9697
VL - 957
JO - Science of the Total Environment
JF - Science of the Total Environment
M1 - 176842
ER -